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Polydimethylsiloxane (PDMS) and poly(3,4-ethylene dioxythiophene):poly(4-styrene-sulfonate) (PEDOT:PSS) composites were tested to determine their suitability for charging small-scale batteries in conjunction with a piezoelectric actuator as an energy harvester. Two different PEDOT:PSS patterns (zigzag and serpentine) were tested, and the maximum DC voltage of a system incorporating PEDOT:PSS was determined. The aim of this work is to study the effect of soft corners in the electrical routing of aircraft and IoT sensors. The zigzag and serpentine patterns were considered for this study because of their simplicity in design. Without the polymer, 2.3 V was produced by the actuator, while adding PEDOT:PSS resulted in the voltage being reduced to 1.7 V. The piezoelectric actuator was connected to a 3.6 V rechargeable Li-ion battery, and the battery's voltage was recorded over 1 h. The voltage from the piezoelectric actuator was 3.8 V. Without PEDOT:PSS, the battery was charged to a maximum of 3 V. Adding the PEDOT:PSS to the circuit reduced the maximum charge to a voltage of 2 V. The results indicate that while PEDOT:PSS composites can be used in conjunction with piezoelectric energy harvesters, more work is still needed to optimize the system to increase efficiency and charging rates.