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Direct ammonia and dihydroxyacetone production in an unbiased photoelectrochemical cell

Author(s): Guo X; Gao RT; Ren S; Nguyen NT; Chen H; Wu L; Wang L;

Photoelectrochemical production of ammonia usually suffers from a low solar-to-ammonia efficiency and a high overpotential, which influences the bias-free operation of sustainable photoelectrochemistry. Herein, we realize solar-driven ammonia production from waste nitrate by constructing copper-osmium catalysts deposited on the Sb2(S,Se)3 semiconductor, e ...

Article GUID: 40617832


Electrochemical Nitrate Reduction to Ammonia on AuCu Single-atom Alloy Aerogels under Wide Potential Window

Author(s): Yu J; Gao RT; Guo X; Nguyen NT; Wu L; Wang L;

Electrocatalytic nitrate reduction to ammonia (NO3RR) is very attractive for nitrate removal and ammonia production in industrial processes. However, the nitrate reduction reaction is characterized by intense hydrogen competition at strong reduction potentials, which greatly limits the Faraday efficiency at strong reduction potentials. Herein, we reported ...

Article GUID: 39264141


Dynamic semiconductor-electrolyte interface for sustainable solar water splitting over 600 hours under neutral conditions

Author(s): Gao RT; Nguyen NT; Nakajima T; He J; Liu X; Zhang X; Wang L; Wu L;

Photoelectrochemical (PEC) water splitting that functions in pH-neutral electrolyte attracts increasing attention to energy demand sustainability. Here, we propose a strategy to in situ form a NiB layer by tuning the composition of the neutral electrolyte with the additions of nickel and borate species, which improves the PEC performance of the BiVO4 phot ...

Article GUID: 36598972


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